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Deamidation: difference between revisions

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Revision 7 — 06:26, 21 Dec 2024
Areapercent_Ayo (talk)
add the cross-link to the compendial chapter
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Revision 8 — 23:52, 3 Jan 2025
StubSorterBot (talk)
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20Rate rises with pH above about 6, with temperature, and with the flexibility of the local backbone. The Asn-Gly context is the fastest by a wide margin; Asn-Ser and Asn-His are also comparatively fast. Glutamine deamidates by the same mechanism but far more slowly, because the corresponding intermediate is a six-membered ring.{{r|manning2010}}20Rate rises with pH above about 6, with temperature, and with the flexibility of the local backbone. The Asn-Gly context is the fastest by a wide margin; Asn-Ser and Asn-His are also comparatively fast. Glutamine deamidates by the same mechanism but far more slowly, because the corresponding intermediate is a six-membered ring.{{r|manning2010}}
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+22== Detection ==
+23Chromatographically, deamidated species usually elute slightly earlier than the parent on [[Reverse-phase HPLC|reverse phase]] and are better resolved by ion-exchange, which separates on the charge difference that deamidation creates.{{r|usp1503}}
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+25By mass spectrometry, the +0.984 Da shift requires high-resolution instrumentation to see on a peptide of a few kilodaltons. On a quadrupole instrument a deamidated peptide is indistinguishable from its parent, and a certificate reporting "observed mass matches calculated" from such an instrument has not excluded it.{{r|manning2010}}
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22== References ==27== References ==
23{{reflist}}28{{reflist}}