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Bacterial endotoxin test (revision 9)

Old revision·13:37, 20 Nov 2024·KarlFischerKit

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Bacterial endotoxin test
Also calledLAL test, BET
DetectsLipopolysaccharide from Gram-negative bacterial cell walls
Compendial chapterUSP General Chapter 85
UnitsEndotoxin units per mg or per mL (EU)
Analytical method infobox · conventions

The bacterial endotoxin test detects lipopolysaccharide, a component of the outer membrane of Gram-negative bacteria that provokes a febrile response when introduced parenterally. The test exploits a clotting cascade in amoebocyte lysate derived from horseshoe crab blood, which is activated by picogram quantities of endotoxin.[1]

Endotoxin is not a living organism and is not removed by sterilisation. A preparation can be sterile and pyrogenic at the same time: autoclaving kills bacteria but leaves their lipopolysaccharide intact and biologically active. Endotoxin is the commonest but not the only pyrogen, and a separate rabbit pyrogen test exists for the wider class.[2] This is why endotoxin and sterility are separate determinations answering separate questions.[1]

Results are expressed in endotoxin units, normalised to mass for a drug substance or to volume for a solution. Compendial limits for parenteral products are calculated from the maximum dose, and a research-chemical certificate reporting an endotoxin figure without the basis of normalisation is difficult to interpret.[3]

Methods

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Three variants are recognised. The gel-clot method observes whether a firm clot forms at a given dilution and gives a limit result rather than a number. The turbidimetric method follows the increase in turbidity as the cascade proceeds and is quantitative. The chromogenic method measures release of a coloured product from a synthetic substrate and is also quantitative.[1]

Recombinant factor C assays, which use a recombinant version of the initiating enzyme rather than crab-derived lysate, have been introduced and are increasingly accepted. They avoid the animal-derived reagent and are more specific, since they respond only to endotoxin and not to β-glucans.

Interference is the routine difficulty. Sample matrices can enhance or inhibit the cascade, so a validated method includes a positive product control demonstrating recovery of a known spike. A result reported without evidence that interference was assessed is not fully interpretable.[1]

References

  1. ^ a b c d United States Pharmacopeia, General Chapter <85>, Bacterial Endotoxins Test.
  2. ^ United States Pharmacopeia, General Chapter <151>, Pyrogen Test.
  3. ^ United States Pharmacopeia, General Chapter <1503>, Quality Attributes of Synthetic Peptide Drug Substances.